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The Xenon-Argon Technology (X-ArT) Collaboration presents a study on the dynamics of pure and xenon-doped liquid argon (LAr) scintillation. Using two types of silicon photomultipliers sensitive to different wavelength ranges, we provide evidence in favor of a contribution from long-lived ( $>10\mathrm{\mu }\mathrm{s}$) extreme ultraviolet (EUV) lines emitted from argon atomic states, which enhances the light yield. This component is present in both pure and xenon-doped LAr, becoming more pronounced at higher xenon concentrations, where it complements the traditional collisional energy transfer process. To explain this mechanism, we develop a comprehensive model of the Xe-doped LAr scintillation process that integrates both collisional and radiative contributions. Additionally, we investigate how xenon doping affects LAr scintillation light yield and pulse shape discrimination. Finally, we hypothesize that the EUV component may explain the emission of spurious electrons, a known challenge in light dark matter searches using noble liquids. By characterizing the scintillation dynamics in Xe-doped LAr, identifying the long-lived EUV component, and exploring the potential origin of spurious electrons, this work lays the groundwork for optimizing detector performance and advancing the design and sensitivity of future noble liquid particle detectors. Published by the American Physical Society2025 

The existence of dark matter in the universe is inferred from abundant astrophysical and cosmological observations. The Global Argon Dark Matter Collaboration (GADMC) aims to perform the searches for dark matter in the form of weakly interacting massive particles (WIMPs), whose collisions with argon nuclei would produce nuclear recoils with tens of keV energy. Argon has been considered an excellent medium for the direct detection of WIMPs as argon-based scintillation detectors can make use of pulse shape discrimination (PSD) to separate WIMP-induced nuclear recoil signals from electron recoil backgrounds with extremely high efficiency. However, argon-based direct dark matter searches must confront the presence of intrinsic³⁹Ar as the predominant source of electron recoil backgrounds (it is a beta-emitter with an endpoint energy of 565 keV and half-life of 269 years). Even with PSD, the³⁹Ar activity in atmospheric argon (AAr), mainly produced and maintained by cosmic ray-induced nuclear reactions, limits the ultimate size of argon-based detectors and restricts their ability to probe very-low-energy events. The discovery of argon from deep underground wells with significantly less³⁹Ar than that in AAr was an important step in the development of direct dark matter detection experiments using argon as the active target. Thanks to pioneering research and successful R&D, in 2012, the first 160 kg batch of underground argon (UAr) was extracted from a CO₂well in Cortez, Colorado. The DarkSide-50 experiment at the Gran Sasso National Laboratory (LNGS) in Italy, the first liquid argon detector ever operated with a UAr target, demonstrated a ∼ 1,400 suppression of the³⁹Ar activity with respect to the atmospheric argon. An even larger suppression is expected for⁴²Ar (another intrinsic beta-emitter with the⁴²K daughter isotope, also a beta-emitter) as its production is expected mainly in the upper atmosphere. Following the results of DarkSide-50, the GADMC initiated the UAr project for extraction from underground and cryogenic purification of 100 t of argon to be used as a target in the next-generation experiment DarkSide-20k. This paper contains a description of the Urania Plant in Cortez, Colorado, where UAr is extracted; the Aria Plant in Sardinia, Italy, an industrial-scale plant comprising a 350-m state-of-the-art cryogenic isotopic distillation column, designed for further purification of the extracted argon and further reduction of the isotopic abundance of³⁹Ar; and DArT, a facility for UAr radiopurity qualification at the Canfranc Underground Laboratory (LSC), Spain. Moreover, the high radiopurity of UAr leads to other possible applications, for instance, for those neutrinoless double-beta decay experiments using argon as shielding material or, more generally, for all those activities on argon-based detectors in high-energy physics or nuclear physics, which will be briefly discussed. 

SiPM-based readouts are becoming the standard for light detection in particle detectors given their superior resolution and ease of use with respect to vacuum tube photo-multipliers. However, the contributions of noise detection such as the dark rate, cross-talk, and after-pulsing (AP) may significantly impact their performance. In this work, we present the development of highly reflective single-phase argon chambers capable of displaying light yields up to 32 photo-electrons per keV, with approximately 12 being primary photo-electrons generated by the argon scintillation, while the rest are accounted by optical cross-talk. Furthermore, the presence of compound processes results in a generalized Fano factor larger than 2 already at an over-voltage of 5 V. Finally, we present a parametrization of the optical cross-talk for the FBK NUV-HD-Cryo SiPMs at 87 K that can be extended to future detectors with tailored optical simulations. 

Borexino could efficiently distinguish between $\alpha$and $\beta$radiation in its liquid scintillator by the characteristic time profile of its scintillation pulse. This $\alpha /\beta$discrimination, first demonstrated on the ton scale in the counting test facility prototype, was used throughout the lifetime of the experiment between 2007 and 2021. With this method, the $\alpha$events are identified and subtracted from the solar neutrino events similar to $\beta$. This is particularly important in liquid scintillators, as the $\alpha$scintillation is strongly quenched. In Borexino, the prominent ${}^{210}\mathrm{Po}$decay peak was a background in the energy range of electrons scattered from ${}^7\mathrm{Be}$solar neutrinos. Optimal $\alpha /\beta$discrimination was achieved with a , with a higher ability to leverage the timing information of the scintillation photons detected by the photomultiplier tubes. An event-by-event, high efficiency, stable, and uniform pulse shape discrimination was essential in characterizing the spatial distribution of background in the detector. This benefited most Borexino measurements, including solar neutrinos in the $pp$chain and the first direct observation of the CNO cycle in the Sun. This paper presents key milestones in $\alpha /\beta$discrimination in Borexino as a term of comparison for current and future large liquid scintillator detectors. Published by the American Physical Society2024 

Abstract Directional sensitivity to nuclear recoils would provide a smoking gun for a possible discovery of dark matter in the form of WIMPs (Weakly Interacting Massive Particles). A hint of directional dependence of the response of a dual-phase argon Time Projection Chamber (TPC) was found in the SCENE experiment. Given the potential importance of such a capability in the framework of dark matter searches, a new dedicated experiment, ReD (Recoil Directionality), was designed by the Global Argon Dark Matter Collaboration, in order to scrutinise this hint. A small dual-phase argon TPC was irradiated with neutrons produced by the p(⁷Li,⁷Be)n reaction using the 15 MV TANDEM accelerator of the INFN - Laboratori Nazionali del Sud, Catania, Italy, so as to produce argon nuclear recoils in the range (20 - 100) keV of interest for dark matter searches. Energy and direction of nuclear recoils are inferred by the detection of the elastically-scattered neutron by a set of scintillation detectors. Events were selected by gating of the associated⁷Be, which is detected by a telescope of Si detectors. 

Abstract The scintillation time response of liquid argon has a key role in the discrimination of electronic backgrounds in dark matter search experiments. However, its extraordinary rejection power can be affected by various detector effects such as the delayed light emission of TetraPhenyl Butadiene, the most commonly used wavelength shifter, and the electric drift field applied in Time Projection Chambers. In this work, we characterized the TetraPhenyl Butadiene delayed response and the dependence of the pulse shape discrimination on the electric field, exploiting the data acquired with the ARIS, a small-scale single-phase liquid argon detector exposed to monochromatic neutron and gamma sources at the ALTO facility of IJC Lab in Orsay. 

Abstract In this work we will document the design and the performances of a SiPM-based photo-detector with a surface area of 100 cm 2 conceived to operate as a replacement for PMTs. The signals from 94 SiPMs are summed up to produce an aggregated output that exhibits in liquid nitrogen a dark count rate (DCR) lower than 100 cps over the entire surface, a signal to noise ratio better than 13, and a timing resolution better than 5.5 ns. The module feeds about 360 mW at 5 V with a dynamic range in excess of 500 photo-electrons on a 100 Ω differential line. The unit can also operate at room temperature, at the cost of an increase of DCR to 10 8 cps.